国际清洁环境能源期刊
每年出版 8 期
ISSN 打印: 2150-3621
ISSN 在线: 2150-363X
SJR:
0.597
SNIP:
1.456
CiteScore™::
3.7
H-Index:
18
Indexed in
A NEW ROUTE OF HCN FORMATION VIA N2O IN GASEOUS HYDROCARBON FLAMES
卷 5,
册 3, 2004,
13 pages
DOI: 10.1615/InterJEnerCleanEnv.v5.i3.80
摘要
The formation of HCN in flames via N2O reactions with CHi radicals proposed by Gradon (2001) and elaborated later (Tomeczek and Gradon, 2003) into a form of elementary step reactions is tested for rich and lean gaseous premixed CH4/air flames. The new route to HCN is thermodynamically more probable than the Fenimore direct reactions of N2 with CHi radicals. To meet the observed NO formation rates, a set of six reactions is proposed:
N2O + CH3 ⇔ CH2NH + NO,
N2O + CH3 ⇔ CH3O + N2,
CH2NH + H ⇔ H2CN + H2,
CH2NH + O ⇔ H2CN + OH,
H2CN + H ⇔ HCN + H2,
H2CN + O ⇔ HCN + OH.
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