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International Journal of Energetic Materials and Chemical Propulsion
ESCI SJR: 0.149 SNIP: 0.16 CiteScore™: 0.29

ISSN Imprimer: 2150-766X
ISSN En ligne: 2150-7678

International Journal of Energetic Materials and Chemical Propulsion

DOI: 10.1615/IntJEnergeticMaterialsChemProp.v6.i2.60
pages 213-228

PHYSICAL AND CHEMICAL PROCESSES GOVERNING THE COMBUSTION OF BINARY COMPOSITIONS OF AMMONIUM DINITRAMIDE WITH GLYCIDYLAZIDEPOLYMER

Valery P. Sinditskii
Department of Chemical Engineering, Mendeleev University of Chemical Technology, Moscow, 125047, Russia
Viacheslav Yu. Egorshev
Department of Chemical Engineering, Mendeleev University of Chemical Technology, 9 Miusskaya Sq., 125047, Moscow, Russia
Anton I. Levshenkov
Department of Chemical Engineering, Mendeleev University of Chemical Technology
Maxim V. Berezin
Department of Chemical Engineering, Mendeleev University of Chemical Technology

RÉSUMÉ

The paper presents a study of the burning behavior and flame structure of compositions consisting of ammonium dinitramide (ADN) and glycidylazidepolymer (GAP). Unlike neat ADN and GAP, the ADN/GAP binary mixtures appeared to burn steadily within the whole pressure interval, showing no breaks on the burning rate vs. pressure dependences. In the low-pressure area, the mixtures burn with rates less than those of pure ADN and exceed it as pressure grows above 10 MPa. In the whole pressure interval, the mixtures burn with the rates higher than those of pure GAP. It was determined on the basis of flame structure investigation that the surface temperature of ADN/GAP mixtures is controlled by the dissociation reaction of ammonium nitrate (AN) formed in the condensed phase during ADN decomposition. Physical and chemical processes responsible for the observed combustion behavior of the mixtures are discussed.


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